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          Institute: MPI für bioanorganische Chemie     Collection: MPI für bioanorganische Chemie     Display Documents



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ID: 677322.0, MPI für bioanorganische Chemie / MPI für bioanorganische Chemie
Reflections on substrate water and dioxygen formation
Authors:Cox, Nicholas; Messinger, Johannes
Language:English
Date of Publication (YYYY-MM-DD):2013
Title of Journal:Biochimica et Biophysica Acta-Bioenergetics
Journal Abbrev.:Biochim. Biophys. Acta-Bioenerg.
Volume:1827
Start Page:1020
End Page:1030
Review Status:Peer-review
Audience:Experts Only
Abstract / Description:This brief article aims at presenting a concise summary of all experimental findings regarding substrate water-binding to the Mn4CaO5 cluster in photosystem II. Mass spectrometric and spectroscopic results are interpreted in light of recent structural information of the water oxidizing complex obtained by X-ray crystallography, spectroscopy and theoretical modeling. Within this framework current proposals for the mechanism of photosynthetic water-oxidation are evaluated. This article is part of a Special Issue entitled: Metals in Bioenergetics and Biomimetics Systems. (C) 2013 Elsevier B.V. All rights reserved.
Free Keywords:Photosystem II; Substrate water binding; Mechanism of water oxidation; Water oxidizing complex (WOC); Oxygen evolving complex (OEC); Mn4CaO5 cluster
External Publication Status:published
Document Type:Article
Communicated by:N. N.
Affiliations:MPI für bioanorganische Chemie
External Affiliations:Messinger, J.; Umea Univ, Chem Biol Ctr KBC, Dept Chem, S-90187 Umea, Sweden.
Identifiers:ISI:000322414300013 [ID No:1]
ISSN:0005-2728 [ID No:2]
DOI:10.1016/j.bbabio.2013.01.013 [ID No:3]
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