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          Institute: MPI für medizinische Forschung     Collection: Jahbruch 2014_archival     Display Documents



ID: 681430.0, MPI für medizinische Forschung / Jahbruch 2014_archival
Time−Resolved Measurement of Interatomic Coulombic Decay in Ne2
Translation of Title:Time−Resolved Measurement of Interatomic Coulombic Decay in Ne2
Authors:Schnorr, Kirsten; Senftleben, Arne; Kurka, Moritz; Rudenko, Artem; Foucar, Lutz; Schmid, Georg; Broska, Alexander; Pfeifer, Thomas; Meyer, Kristina; Anielski, Denis; Boll, Rebecca; Rolles, Daniel; Kübel, Matthias; Kling, Matthias F.; Jiang, Yuhai; Mondal, Subhendu; Tachibana, Tetsuya; Ueda, Kiyoshi; Marchenko, Tatiana; Simon, Mark; Brenner, Günther; Treusch, Rolf; Scheit, Simona; Averbukh, Vitali; Ullrich, Joachim; Schröter, Claus−Dieter; Moshammer, Robert
Language:English
Date of Publication (YYYY-MM-DD):2013-08-27
Title of Journal:Physical Review Letters
Journal Abbrev.:Physical Review Letters
Volume:111
Issue / Number:9
Start Page:1
End Page:5
Sequence Number of Article:093402
Review Status:Peer-review
Audience:Experts Only
Intended Educational Use:No
Abstract / Description:The lifetime of interatomic Coulombic decay (ICD) [L. S. Cederbaum et al., Phys. Rev. Lett. 79, 4778 (1997)] in Ne2 is determined via an extreme ultraviolet pump−probe experiment at the Free−Electron Laser in Hamburg. The pump pulse creates a 2s inner−shell vacancy in one of the two Ne atoms, whereupon the ionized dimer undergoes ICD resulting in a repulsive Ne+(2p−1)−Ne+(2p−1) state, which is probed with a second pulse, removing a further electron. The yield of coincident Ne+−Ne2+ pairs is recorded as a function of the pump−probe delay, allowing us to deduce the ICD lifetime of the Ne+2(2s−1) state to be (150±50)  fs, in agreement with quantum calculations
External Publication Status:published
Document Type:Article
Communicated by:wkaiser
Affiliations:MPI für medizinische Forschung/Abteilung Zellphysiologie
MPI für medizinische Forschung/Abteilung Biomolekulare Mechanismen
MPI für medizinische Forschung/Abteilung Biomolekulare Mechanismen/Coherent diffractive imaging
Identifiers:LOCALID:7967
URI:http%3A%2F%2Fprl.aps.org%2Fpdf%2FPRL%2Fv111%2Fi9%2...
URI:http%3A%2F%2Fprl.aps.org%2Fabstract%2FPRL%2Fv111%2...
DOI:10.1103%2FPhysRevLett.111.093402
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