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          Institute: MPI für medizinische Forschung     Collection: Jahbruch 2014_archival     Display Documents



ID: 681478.0, MPI für medizinische Forschung / Jahbruch 2014_archival
Ultrafast charge rearrangement and nuclear dynamics upon inner−shell multiple ionization of small polyatomic molecules
Translation of Title:Ultrafast charge rearrangement and nuclear dynamics upon inner−shell multiple ionization of small polyatomic molecules
Authors:Erk, Benjamin; Rolles, Daniel; Foucar, Lutz; Rudek, Benedikt; Epp, Sascha W.; Cryle, Max; Bostedt, Christoph; Schorb, Sebastian; Bozek, John D.; Rouzee, Arnaud; Hundertmark, Axel; Marchenko, Tatiana; Simon, Marc; Filsinger, Frank; Christensen, Lauge; De, Shankar; Trippel, Sebastian; Küpper, Jochen; Stapelfeldt, Henrik; Wada, Shinichi; Ueda, Kiyoshi; Swiggers, Michelle L.; Messerschmidt, Marc; Schroeter, Claus−Dieter; Moshammer, Robert; Schlichting, Ilme; Ullrich, Joachim; Rudenko, Artem
Language:English
Date of Publication (YYYY-MM-DD):2013-02-01
Title of Journal:Physical Review Letters
Journal Abbrev.:Phys. Rev. Lett.
Volume:110
Issue / Number:5
Start Page:1
End Page:5
Sequence Number of Article:53003
Review Status:Peer-review
Audience:Experts Only
Intended Educational Use:No
Abstract / Description:Ionization and fragmentation of methylselenol (CH3SeH) molecules by intense (>1017  W/cm2) 5 fs x−ray pulses (ℏω=2  keV) are studied by coincident ion momentum spectroscopy. We contrast the measured charge state distribution with data on atomic Kr, determine kinetic energies of resulting ionic fragments, and compare them to the outcome of a Coulomb explosion model. We find signatures of ultrafast charge redistribution from the inner−shell ionized Se atom to its molecular partners, and observe significant displacement of the atomic constituents in the course of multiple ionization
External Publication Status:published
Document Type:Article
Communicated by:wkaiser
Affiliations:MPI für medizinische Forschung/Abteilung Biophysik
MPI für medizinische Forschung/Abteilung Biomolekulare Mechanismen
MPI für medizinische Forschung/Abteilung Biomolekulare Mechanismen/Cytochrome P450
MPI für medizinische Forschung/Abteilung Biomolekulare Mechanismen/Coherent diffractive imaging
Identifiers:LOCALID:7882
URI:http%3A%2F%2Fprl.aps.org%2Fpdf%2FPRL%2Fv110%2Fi5%2...
URI:http%3A%2F%2Fwww.ncbi.nlm.nih.gov%2Fpubmed%2F23414...
DOI:10.1103%2FPhysRevLett.110.053003
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